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Thermally Controllable Multiple High Harmonics Generation by Phase-Change Materials-Mediated Fano Clusters

机译:用热力可控的多谐波产生   相变材料介导的Fano团簇

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摘要

Substantial enhancement of nonlinear high-order harmonics generation based onFano-resonant nanostructures has received growing interest due to theirpromising potential for developing integrated and advanced next-generationnanophotonic devices. In this study, going beyond conventional subwavelengthstructures, we propose an optothermally functional hetero-metallodielectricasymmetric eight-member octamer cluster composed of a central silicon nanodiskand peripheral disks with a phase-change material (Ge2Sb2Te5). Using fullelectromagnetic calculations, we show that in the amorphous phase of thesurrounding particles, the oligomer acts as an all-dielectric cluster, while inthe crystalline regime, the octamer turns into a hybrid metallodielectricassembly. Exploiting the exquisite ability of supporting distinct Fanolineshapes at different wavelengths depending on the phase of Ge2Sb2Te5, weshowed the generation of both second and third harmonics at amorphous andcrystalline phases of GST nanodisks, respectively with the produced harmonicwavelengths of 425 nm and 317 nm, respectively. Our calculations for thecorresponding conversion efficiencies revealed significant enhancements as{\eta}SHG=0.012% and {\eta}THG=0.0081% for SHG and THG, respectively. Such anexquisite feature of multiresonant optothermally tunable cluster allowsgeneration of several higher-harmonics with distinct intensities using a singlesystem for future photonics applications.
机译:由于其在开发集成和先进的下一代纳米光子器件方面的潜力,基于泛纳共振纳米结构的非线性高阶谐波产生的实质性增强已引起越来越多的关注。在这项研究中,我们超越了常规的亚波长结构,提出了一种光热功能的异金属介电不对称八元八聚体簇,该簇由中心硅纳米盘和具有相变材料(Ge2Sb2Te5)的外围盘组成。使用全电磁计算,我们表明,在周围粒子的非晶相中,低聚物充当全介电团簇,而在结晶状态下,八聚体变成混合金属介电体。利用根据Ge2Sb2Te5的相位支持不同波长的不同Fanoline形状的出色能力,我们展示了GST纳米盘的非晶相和结晶相分别产生二次谐波和三次谐波,产生的谐波波长分别为425 nm和317 nm。我们对相应转换效率的计算表明,SHG和THG分别显着提高{\ eta} SHG = 0.012%和{\ eta} THG = 0.0081%。多谐振光热可调谐簇的这种精妙特征允许使用单个系统为未来的光子学应用生成具有不同强度的几个高次谐波。

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